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Full Record Details
Persistent URL
http://purl.org/net/epubs/work/30362
Record Status
Checked
Record Id
30362
Title
Comparison of Aerosol and Thin Film Spectra of Supercooled Ternary Solution Aerosol
Contributors
RA McPheat (CCLRC Rutherford Appleton Lab.)
,
SF Bass (Oxford U.)
,
DA Newnham (CCLRC Rutherford Appleton Lab.)
,
J Ballard (CCLRC Rutherford Appleton Lab.)
,
JJ Remedios (Oxford U.)
Abstract
Extinction spectra of H2SO4-HNO3-H2O supercooled ternary solution (STS) aerosol particles, fully covering the mid- and near-infrared region from 750 to 13,000 cm-1 (13.9 to 0.7 micron), have been measured in the laboratory using a 75 dm3-volume coolable aerosol cell coupled with a Fourier transform spectrometer. The STS spectra were recorded at temperatures close to those encountered in the polar stratosphere, and were fitted to a spectrum modelled by combining Mie scattering theory and published thin film refractive index data. Good agreement between model and laboratory data was found in the region 1300 - 13,000 cm-1, but significant deviations were found in the region 750 - 1300 cm-1.
Organisation
CCLRC
,
SSTD
Keywords
PSC
,
Physics
,
Chemistry
,
Natural environment
,
STS
,
laboratory
,
aerosol
,
refractive index
Funding Information
Related Research Object(s):
Licence Information:
Language
English (EN)
Type
Details
URI(s)
Local file(s)
Year
Journal Article
J Geophys Res
107, no. d19 (2002): 4371.
doi:10.1029/2001jd000641
2002
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