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Persistent URL http://purl.org/net/epubs/work/39795501
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Record Id 39795501
Title Investigation of ZSM-5 catalysts for dimethylether conversion using inelastic neutron scattering
Contributors
Abstract We report the characterisation of zeolite ZSM-5 catalysts used in the conversion of dimethylether to hydrocarbons. Inelastic neutron scattering spectroscopy, supported by solid state NMR, shows that the more rapid deactivation occurring with dimethylether compared with methanol is associated with the formation of less methylated aromatic coke species and attributed to the lower levels of water present during dimethylether conversion. The ability of inelastic neutron scattering to probe a working catalyst with no sample preparation is demonstrated.
Organisation ISIS , ISIS-TOSCA , ISIS-MERLIN , STFC
Keywords
Funding Information Engineering and Physical Sciences Research Council (EP/K014706/1); Engineering and Physical Sciences Research Council (EP/K014668/1); Engineering and Physical Sciences Research Council (EP/K014854/1); Engineering and Physical Sciences Research Council (EP/K014714/1); Engineering and Physical Sciences Research Council (EP/M013219/1)
Related Research Object(s):
Language English (EN)
Type Details URI(s) Local file(s) Year
Journal Article Appl Catal A Gen 569 (2019): 1-7. https://doi.org/1…j.apcata.2018.10.010 2019
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