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Full Record Details
Persistent URL
http://purl.org/net/epubs/work/65835
Record Status
Checked
Record Id
65835
Title
MnSb_{2}O_{6}: A Polar Magnet with a Chiral Crystal Structure
Contributors
RD Johnson (Oxford U.)
,
K Cao (Oxford U.)
,
LC Chapon (Institut Laue-Langevin)
,
F Fabrizi (Oxford U.)
,
N Perks (Oxford U.)
,
P Manuel (STFC Rutherford Appleton Lab.)
,
JJ Yang (Pohang University of Science and Technology)
,
YS Oh (Rutgers U.)
,
S Cheong (Rutgers U.)
,
PG Radaelli (Oxford U.)
Abstract
Structural and magnetic chiralities are found to coexist in a small group of materials in which they produce intriguing phenomenologies such as the recently discovered Skyrmion phases. Here, we describe a previously unknown manifestation of this interplay in MnSb2O6, a trigonal oxide with a chiral crystal structure. Unlike all other known cases, the MnSb2O6 magnetic structure is based on corotating cycloids rather than helices. The coupling to the structural chirality is provided by a magnetic axial vector, related to the so-called vector chirality. We show that this unique arrangement is the magnetic ground state of the symmetric-exchange Hamiltonian, based on ab initio theoretical calculations of the Heisenberg exchange interactions, and is stabilized by out-of-plane anisotropy. MnSb2O6 is predicted to be multiferroic with a unique ferroelectric switching mechanism.
Organisation
ISIS
,
ISIS-WISH
,
STFC
Keywords
ISIS 2013
Funding Information
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Language
English (EN)
Type
Details
URI(s)
Local file(s)
Year
Journal Article
Phys Rev Lett
111, no. 1 (2013): 017202.
doi:10.1103/PhysRevLett.111.017202
2013
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